Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit
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| Định dạng: | Bài Báo |
| Ngôn ngữ: | English |
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ACS Appl. Nano Mater. 2021
2021
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| Truy cập trực tuyến: | https://pubs.acs.org/doi/10.1021/acsanm.1c00169 https://dlib.phenikaa-uni.edu.vn/handle/PNK/1850 |
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oai:localhost:PNK-18502022-08-17T05:54:41Z Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit Pham, Minh T. Luong, Hoang M. Pham, Huy T. Guin, Tyler Zhao, Yiping George K., Larsen Nguyen, Tho D. ppb limit of detection composite hole arrays magnetic hydride resistance nanonetwork electrical hydrogen sensor Q1 As hydrogen gas increasingly becomes critical as a carbon-free energy carrier, the demand for robust hydrogen sensors for leak detection and concentration monitor will continue to rise. However, to date, there are no lightweight sensors capable of meeting the required performance metrics for the safe handling of hydrogen. Here, we report an electrical hydrogen gas sensor platform based on a resistance nanonetwork derived from Pd-Co composite hole arrays (CHAs) on a glass substrate, which meets or exceeds these metrics. In optimal nanofabrication conditions, a single poly(methyl methacrylate)(PMMA)-coated CHA nanosensor exhibits a response time (t80) of 1.0 s at the lower flammability limit of H2 (40 mbar), incredible sensor accuracy (<1% across 5 decades of H2 pressure), and an extremely low limit of detection (LOD) of <10 ppb at room temperature. Remarkably, these nanosensors are extremely inert against CO and O2 gas interference and display robust long-term stability in air, suffering no loss of performance over 2 months. Additionally, we demonstrate that the unique nanomorphology renders the sensors insensitive to operation voltage/current with diminutive power requirement (∼2 nW) and applied magnetic field (up to 3 kOe), a crucial metric for leak detection and concentration control. 2021-06-18T02:29:50Z 2021-06-18T02:29:50Z 2021 Article Working Paper https://pubs.acs.org/doi/10.1021/acsanm.1c00169 https://dlib.phenikaa-uni.edu.vn/handle/PNK/1850 doi.org/10.1021/acsanm.1c00169 en ACS Appl. Nano Mater. 2021 |
| institution |
Digital Phenikaa |
| collection |
Digital Phenikaa |
| language |
English |
| topic |
ppb limit of detection composite hole arrays magnetic hydride resistance nanonetwork electrical hydrogen sensor |
| spellingShingle |
ppb limit of detection composite hole arrays magnetic hydride resistance nanonetwork electrical hydrogen sensor Pham, Minh T. Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit |
| description |
Q1 |
| author2 |
Luong, Hoang M. |
| author_facet |
Luong, Hoang M. Pham, Minh T. |
| format |
Article |
| author |
Pham, Minh T. |
| author_sort |
Pham, Minh T. |
| title |
Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit |
| title_short |
Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit |
| title_full |
Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit |
| title_fullStr |
Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit |
| title_full_unstemmed |
Pd80Co20 Nanohole Arrays Coated with Poly(methyl methacrylate) for High-Speed Hydrogen Sensing with a Part-per-Billion Detection Limit |
| title_sort |
pd80co20 nanohole arrays coated with poly(methyl methacrylate) for high-speed hydrogen sensing with a part-per-billion detection limit |
| publisher |
ACS Appl. Nano Mater. 2021 |
| publishDate |
2021 |
| url |
https://pubs.acs.org/doi/10.1021/acsanm.1c00169 https://dlib.phenikaa-uni.edu.vn/handle/PNK/1850 |
| _version_ |
1751856253628317696 |
| score |
8.891145 |